Polariton-mediated Raman scattering in microcavities: A Green's function approach

We present calculations of the intensity of polariton-mediated inelastic light scattering in semiconductor microcavities within a Green's function framework. In addition to reproducing the strong coupling of light and matter, this method also enables the inclusion of damping mechanisms in a consistent way. Our results show excellent agreement with recent Raman scattering experiments.Comment: 6 pages, 1 figur

Cavity polariton optomechanics: Polariton path to fully resonant dispersive coupling in optomechanical resonators

Resonant photoelastic coupling in semiconductor nanostructures opens new perspectives for strongly enhanced light-sound interaction in optomechanical resonators. One potential problem, however, is the reduction of the cavity Q-factor induced by dissipation when the resonance is approached. We show in this letter that cavity-polariton mediation in the light-matter process overcomes this limitation allowing for a strongly enhanced photon-phonon coupling without significant lifetime reduction in the strongly-coupled regime. Huge optomechanical coupling factors in the PetaHz/nm range are envisaged, three orders of magnitude larger than the backaction produced by the mechanical displacement of the cavity mirrors.Comment: 6 pages, 4 figure

Dispersion and damping of multi-quantum well polaritons from resonant Brillouin scattering by folded acoustic modes

We report on confined exciton resonances of acoustic and folded acoustic phonon light scattering in a GaAs/AlAs multi-quantum-well. Significant variations of the line shifts and widths are observed across the resonance and quantitatively reproduced in terms of the polariton dispersion. This high resolution Brillouin study brings new unexpectedly detailed informations on the polariton dynamics in confined systems

Has the chemical contribution a secondary role in SERS?

It is an established understanding that the electromagnetic contribution (the plasmon-mediated enhancement of the laser and scattered local electromagnetic fields) is the main actor in Surface Enhanced Raman Scattering (SERS), with the so-called chemical (molecule-related) contribution assuming only, if any, a supporting role. The conclusion of our comprehensive resonant study of a broad range of nanosphere lithography based metallic substrates, with covalently attached 4-mercaptobenzoic acid monolayers used as probe (molecules non-resonant in solution), is that this accepted understanding needs to be revised. We present a detailed resonant SERS study of Metal-film over nanosphere (MFON) substrates done both by scanning the laser wavelength, and by tuning the plasmon response through the nanosphere diameter. Far and local field properties are characterized through measures of optical reflectivity and SERS efficiency, respectively, and are supported by numerical simulations. We demonstrate that the SERS efficiency depends indeed on the electromagnetic mechanism, determined by the plasmonic response of the system, but we observe that it is also strongly defined by a chemical resonant contribution related to a metal-to-ligand electronic transition of the covalently bound probe molecule. Optimum amplification occurs when the plasmon modes intersect with the ligand-to-metal chemical resonance, contributing synergically both mechanisms together. The same general trend is observed for other nanosphere lithography based substrates, including sphere-segment void cavities and hexagonally ordered triangular nanoparticles, using both Ag or Au as the plasmonic metal, and also with a commercial substrate (Klarite). We conclude that a deep understanding of both the electromagnetic and chemical mechanisms is necessary to fully exploit these substrates for analytical applications

Uncoupled excitons in semiconductor microcavities detected in resonant Raman scattering

We present an outgoing resonant Raman-scattering study of a GaAs/AlGaAs based microcavity embedded in a p-i-n junction. The p-i-n junction allows the vertical electric field to be varied, permitting control of exciton-photon detuning and quenching of photoluminescence which otherwise obscures the inelastic light scattering signals. Peaks corresponding to the upper and lower polariton branches are observed in the resonant Raman cross sections, along with a third peak at the energy of uncoupled excitons. This third peak, attributed to disorder activated Raman scattering, provides clear evidence for the existence of uncoupled exciton reservoir states in microcavities in the strong-coupling regime

Cavity Optomechanics with a Laser Engineered Optical Trap

Laser engineered exciton-polariton networks could lead to dynamically configurable integrated optical circuitry and quantum devices. Combining cavity optomechanics with electrodynamics in laser configurable hybrid designs constitutes a platform for the vibrational control, conversion, and transport of signals. With this aim we investigate 3D optical traps laser-induced in quantum-well embedded semiconductor planar microcavities. We show that the laser generated and controlled discrete states of the traps dramatically modify the interaction between photons and phonons confined in the resonators, accessing through coupling of photoelastic origin $g_\mathrm{0}/2\pi\sim 1.7$ MHz an optomechanical cooperativity $C>1$ for mW excitation. The quenching of Stokes processes and double-resonant enhancement of anti-Stokes ones involving pairs of discrete optical states in the side-band resolved regime, allows the optomechanical cooling of 180 GHz bulk acoustic waves, starting from room temperature down to $\sim120$ K. These results pave the way for dynamical tailoring of optomechanical actuation in the extremely-high-frequency range (30-300 GHz) for future network and quantum technologies.Comment: 22 pages, 14 figure